The actor, 46, and his 38-year-old hit-making partner were seen taking in the sites around the venue before settling in to watch British player Jodie Burrage as she lost her slot in the competition.
During their day out at the All England Lawn Tennis Club, the A-list pairing snapped numerous selfies and showered each other with loving kisses and cuddles.
Orlando looked dapper in a navy-checked two-piece suit and black brogue shoes that he wore over a pin-stripped blue shirt and dark tie in the same colour.
He kept the sun off his face with a pair of blue-tinted sunglasses and appeared with a bearded face for the tennis.
His partner Katy was a vision in a matching navy Bardot top that she sported with a white silk midi skirt and stiletto heels.
She slicked her dark hair back from her face in a vintage-style fringe and half-up-half-down ponytail and accessorised with a polka-dot neck scarf.
Eager to get inside, the stars patiently waited for their turn to take their seats and made it just in time for the roof to open on Centre Court after rain showers caused it to close.
They were in the stands to witness Britain’s hopeful Jodie tragically lose out on another chance to play as she was defeated by Daria Kasatkina.
Katy and Orlando were not the only celebrities out in full force to catch a spot of tennis on the third day of the much-loved tournament.
David Beckham, 48, treated his mum to a seat in the Royal Box and watched the same match with tense expressions.
The former footballer was dressed well for the occasion, putting on a beige suit jacket, cream chinos and a crisp white shirt.
He jazzed up his ensemble with a brown patterned pocket square and a matching tie and wore a lavish watch around his wrist.
The star’s mother Sandra Beckham matched the grass in a pastel green blazer that she draped over the top of a silk shirt in the same colour.
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